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Synthesis of peri-annelated heterocyclic systems based on 3-substituted 1-aryl-4,6-dinitro-1H-indazoles Full article

Journal Russian Chemical Bulletin
ISSN: 1573-9171 , E-ISSN: 1066-5285
Output data Year: 2003, Volume: 52, Number: 8, Pages: 1777-1781 Pages count : 5 DOI: 10.1023/a:1026056704860
Authors Starosotnikov A.M. 1 , Lobach A.V. 1 , Vinogradov V.M. 1 , Shevelev S.A. 1
Affiliations
1 N.D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, Moscow (Russian Federation)

Abstract: A method for the synthesis of peri-annelated trinuclear heterocycles, including 14π-electron heteroaromatic systems, namely, 1H-thiopyrano[4,3,2-cd]indazoles and 1,5-dihydropyrazolo[3,4,5-de]cinnolines, from 3-R-1-aryl-4,6-dinitro-1H-indazoles was developed. The method is based on the high mobility of the NO2 group in position 4 and consists of either selective nucleophilic substitution of the 4-NO2 group on treatment with the HSCH2CO2Me—K2CO3 system followed by intramolecular cyclization of the resulting sulfide (R = CHO) or the corresponding sulfone (R = CN) formed upon its oxidation or direct intramolecular substitution of the 4-NO2 group (R = CH=NNHPh).
Cite: Starosotnikov A.M. , Lobach A.V. , Vinogradov V.M. , Shevelev S.A.
Synthesis of peri-annelated heterocyclic systems based on 3-substituted 1-aryl-4,6-dinitro-1H-indazoles
Russian Chemical Bulletin. 2003. V.52. N8. P.1777-1781. DOI: 10.1023/a:1026056704860 WOS Scopus OpenAlex
Identifiers:
Web of science: WOS:000186446500019
Scopus: 2-s2.0-0347003372
OpenAlex: W2951720351
Citing:
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OpenAlex 5
Scopus 4
Web of science 5
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