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Synthesis of 4,6-dinitro-3-R-benzo[d]isoxazoles and their transformations under the action of nucleophiles Full article

Journal Russian Chemical Bulletin
ISSN: 1573-9171 , E-ISSN: 1066-5285
Output data Year: 2001, Volume: 50, Number: 3, Pages: 464-469 Pages count : 6 DOI: 10.1023/a:1011313324497
Authors Vinogradov V.M. 1 , Dalinger I.L. 1 , Starosotnikov A.M. 1 , Shevelev S.A. 1
Affiliations
1 N. D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, 47 Leninsky prosp., 119992, Moscow, Russian Federation

Abstract: A new procedure was developed for the preparation of 4,6-dinitro-3-R-benzo[d]isoxazoles (R are derivatives of the aldehyde group) based on 2,4,6-trinitrophenylacetaldehyde. The resulting compounds are characterized by the regiospecific substitution of the nitro group at position 4 under the action of anionic nucleophiles RS–, RO–, F–, or N3 –, which allowed the development of a new method for the preparation of previously unknown 4-Nu-6-nitro-3-R-benzo[d]isoxazoles (Nu is the residue of a nucleophile). At the same time, oxidative nucleophilic substitution under the action of anions of some β-dicarbonyl compounds leads to the replacement of the hydrogen atom at position 7 with the corresponding C-nucleophiles.
Cite: Vinogradov V.M. , Dalinger I.L. , Starosotnikov A.M. , Shevelev S.A.
Synthesis of 4,6-dinitro-3-R-benzo[d]isoxazoles and their transformations under the action of nucleophiles
Russian Chemical Bulletin. 2001. V.50. N3. P.464-469. DOI: 10.1023/a:1011313324497 WOS Scopus OpenAlex
Identifiers:
Web of science: WOS:000170218100020
Scopus: 2-s2.0-0035537458
OpenAlex: W2996557919
Citing:
DB Citing
OpenAlex 16
Scopus 20
Web of science 31
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